Volume 1 Issue 1
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Li Peng, Kim Hun, Ming Jun, Jung Hun-Gi, Belharouak Ilias, Sun Yang-Kook. Quasi-compensatory effect in emerging anode-free lithium batteries[J]. eScience, 2021, 1(1): 3-12. doi: 10.1016/j.esci.2021.10.002
Citation: Li Peng, Kim Hun, Ming Jun, Jung Hun-Gi, Belharouak Ilias, Sun Yang-Kook. Quasi-compensatory effect in emerging anode-free lithium batteries[J]. eScience, 2021, 1(1): 3-12. doi: 10.1016/j.esci.2021.10.002
shu

Quasi-compensatory effect in emerging anode-free lithium batteries

doi: 10.1016/j.esci.2021.10.002
  • a.

    Department of Energy Engineering, Hanyang University, Seoul 04763, Republic of Korea

  • b.

    State Key Laboratory of Rare Earth Resource Utilization, Changchun Institute of Applied Chemistry, CAS, Changchun 130022, China

  • c.

    School of Applied Chemistry and Engineering, University of Science and Technology of China, Hefei 230026, China

  • d.

    Center for Energy Storage Research, Korea Institute of Science and Technology, Seoul 02792, Republic of Korea

  • e.

    Division of Energy & Environment Technology, Korea University of Science and Technology, Daejeon 34113, Republic of Korea

  • f.

    Electrification and Energy Infrastructure Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831, United States

  • g.

    Bredesen Center for Interdisciplinary Research and Graduate Education, University of Tennessee, Knoxville, TN 37996, United States

More Information
  • Corresponding author: E-mail addresses: hungi@kist.re.kr (H.-G. Jung); E-mail addresses: yksun@hanyang.ac.kr (Y.-K. Sun)
  • Received Date: 2021-08-05
  • Revised Date: 2021-09-22
  • Accepted Date: 2021-10-04
    • Available Online: 2021-10-06
    Abstract
  • As electric vehicle (EV) sales grew approximately 50% year-over-year, surpassing 3.2 million units in 2020, the "roaring era" of EV is around the corner. To meet the increasing demand for low cost and high energy density batteries, anode-free configuration, with no heavy and voluminous host material on the current collector, has been proposed and further investigated. Nevertheless, it always suffers from several nonnegligible "bottlenecks", such as fragile solid electrolyte interface, deteriorated cycling reversibility, and uncontrolled dendrite formation. Inspired by the "compensatory effect" of some disabled people with other specific functions strengthened to make up for their inconvenience, corresponding quasi-compensatory measures after anode removal, involving dimensional compensation, SEI robustness compensation, lithiophilicity compensation, and lithium source compensation, have been carried out and achieved significant battery performance enhancement. In this review, the chemistry, challenges, and rationally designed "quasi-compensatory effect" associated with anode-free lithium-ion battery are systematically discussed with several possible R & D directions that may aid, direct, or facilitate future research on lithium storage in anode-free configuration essentially emphasized.
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