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Article Navigation >  eScience  > 2021  >  1(2): 141-162
Huang Aoming, Ma Yanchen, Peng Jian, Li Linlin, Chou Shu-lei, Ramakrishna Seeram, Peng Shengjie. Tailoring the structure of silicon-based materials for lithium-ion batteries via electrospinning technology[J]. eScience, 2021, 1(2): 141-162. doi: 10.1016/j.esci.2021.11.006
Citation: Huang Aoming, Ma Yanchen, Peng Jian, Li Linlin, Chou Shu-lei, Ramakrishna Seeram, Peng Shengjie. Tailoring the structure of silicon-based materials for lithium-ion batteries via electrospinning technology[J]. eScience, 2021, 1(2): 141-162. doi: 10.1016/j.esci.2021.11.006
shu

Tailoring the structure of silicon-based materials for lithium-ion batteries via electrospinning technology

doi: 10.1016/j.esci.2021.11.006
  • a.

    College of Materials Science and Technology, Nanjing University of Aeronautics and Astronautics, Nanjing, 210016, China

  • b.

    Institute for Superconducting and Electronic Materials, Australian Institute for Innovative Materials, University of Wollongong Innovation Campus, Squires Way, North Wollongong, NSW, 2522, Australia

  • c.

    Center for Nanofibers and Nanotechnology, Department of Mechanical Engineering, National University of Singapore, Singapore, 117576, Singapore

More Information
  • Corresponding author: E-mail address: pengshengjie@nuaa.edu.cn (S. Peng)
  • Received Date: 2021-08-03
  • Revised Date: 2021-10-27
  • Accepted Date: 2021-11-30
    • Available Online: 2021-12-04
    Abstract
  • Silicon (Si) is one of the most promising anode materials for the next generation of lithium-ion battery (LIB) due to its high specific capacity, low lithiation potential, and natural abundance. However, the huge variation in volume during the storage of lithium, along with the low conductivity of element, are the main factors hindering its commercial application. Designing micro–nano structures as well as composites of heterogeneous materials have proven to be effective strategies to overcome these issues. Electrospinning technology is an affordable and scalable method for easily constructing a unique hierarchical micro–nano structure while realizing composites of heterogeneous materials. So far, many efforts have been made to solve the problems of Si-based anodes with general electrospinning. This review considers the technical fundamental and design strategies for electrospun Si-based nanofibers, including preparation processes, structural engineering, and lithium storage performance. The structure–performance relationship of various materials and the effects of compositing with heterogeneous materials are explored in detail. Finally, the remaining challenges are discussed, along with directions for future research. This review will provide inspiration for researchers in the design and manufacture of electrospun Si-based nanofibers for LIBs.
    • ● The application in lithium-ion battery anode is discussed.
    ● The synthetic routes of electrospun silicon-based nanofibers are described.
    ● The challenge and directions for future research is proposed.
    ● The structure design strategy is reviewed.
    Abbreviations: ALD, Atomic layer deposition; CNF, Carbon nanofibers; CNT, Carbon nanotubes; CVD, Chemical vapor deposition; DMF, N, N-dimethylformamide; ICE, Initial Coulombic efficiency; LIB, Lithium-ion battery; NP, Nanoparticles; PAA, Poly(acrylic acid); PAN, Polyacrylonitrile; PLLA, Poly(L-lactic acid); PMMA, Poly(methyl methacrylate); PPy, Polypyrrole; PS, Polystyrene; PVA, Poly(vinyl alcohol); PVP, Poly(vinylpyrrolidone); REF, Reference; SEI, Solid electrolyte interphase; SEM, Scanning electron microscope; TEM, Transmission electron microscope; TEOS, Tetraethoxysilane.
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