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Zhu Yan-Fang, Xiao Yao, Dou Shi-Xue, Kang Yong-Mook, Chou Shu-Lei. Spinel/Post-spinel engineering on layered oxide cathodes for sodium-ion batteries[J]. eScience, 2021, 1(1): 13-27. doi: 10.1016/j.esci.2021.10.003
Citation: Zhu Yan-Fang, Xiao Yao, Dou Shi-Xue, Kang Yong-Mook, Chou Shu-Lei. Spinel/Post-spinel engineering on layered oxide cathodes for sodium-ion batteries[J]. eScience, 2021, 1(1): 13-27. doi: 10.1016/j.esci.2021.10.003
shu

Spinel/Post-spinel engineering on layered oxide cathodes for sodium-ion batteries

doi: 10.1016/j.esci.2021.10.003
  • a.

    Institute for Carbon Neutralization, College of Chemistry and Materials Engineering, Wenzhou University, Wenzhou, Zhejiang 325035, China

  • b.

    Australian Institute for Innovative Materials, Institute for Superconducting and Electronic Materials, University of Wollongong, Innovation Campus, Squires Way, North Wollongong, NSW 2522, Australia

  • c.

    Department of Materials Science and Engineering, Korea University, Seoul 02841, Republic of Korea

  • d.

    KU-KIST Graduate School of Converging Science and Technology, Korea University, Seoul 02841, Republic of Korea

More Information
  • Corresponding author: E-mail addresses: dake1234@korea.ac.kr (Y.-M. Kang); E-mail addresses: chou@wzu.edu.cn (S.-L. Chou)
  • Received Date: 2021-06-11
  • Revised Date: 2021-09-06
  • Accepted Date: 2021-10-07
    • Available Online: 2021-10-09
    Abstract
  • Sodium-ion batteries (SIBs) have attracted much scientific interest for use in large-scale energy storage systems because sodium is cheaper than lithium. However, the large radius of Na+ and barriers to Na+ transport result in sluggish kinetics and complicated structural distortion, leading to unsatisfactory rate capability and poor cycling stability. It therefore is essential to develop an electrode with enhanced kinetics and a stable structure during cycling to improve SIB performance. Among the various layered oxide cathodes, those with a spinel-like structure could play an important role in boosting electron transport because of their excellent intrinsic conductivity, including by coordinating with Na + insertion/extraction. Moreover, thanks to the inherent high stability of the spinel-like phase, it could function as a stabilizer for host cathode structures. This review summarizes recent advances in spinel engineering on layered oxide cathodes to boost Na+ transport kinetics and provide structural stability to achieve high-performance SIBs, focusing particularly on post-spinel structures, layered oxide integrated spinel-like structures, and spinel transitions. The insights proposed in this review will be useful for guiding rational structural engineering and design to drive the development of new materials and chemistries in Na-based electrode materials.
    • # Dr. Y.-F. Zhu and Dr. Y. Xiao contributed equally to this work.
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